EVALUATION OF THE PHYSICOCHEMICAL PARAMETERS, BIOSURFACTANT PRODUCTION AND METAGENOMIC ANALYSIS OF HYDROCARBON POLLUTED SOIL.

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ABSTRACT

The evaluation of the physicochemical parameters, biosurfactant production and metagenomic analysis of hydrocarbon polluted soil in Opuama, Ogini, Oteghele, Transforcados pipeline and Transforcados right of way sites located at Isoko North, Warri North and South LGA of Delta State Nigeria, was carried out using standard microbiological and physicochemical methods. Hydrocarbon utilizing bacteria (HUB), total heterotrophic bacterial count (THB), physicochemical analysis including heavy metals, screening and characterization, optimization of biosurfactant using response surface methodology (RSM) and metagenomic analysis were all carried out.  The DNA of the microorganisms from the soil samples were extracted using ZymoDNA extraction kit, amplified and subjected to next generational sequencing (NGS) on Pacbio SMR sequencing platform. Following NGS, gene calling was performed using freg gene scan and the resulting metagenome were then functionally annotated onto two pipelines namely: cluster of orthology group (COG) and Kyoto encyclopedia of genes and genomes (KEGG) for functional gene analysis. The bacteria screened and characterized for biosurfactant production were Escherichia coliBacillus subtilisEnterobacter aerogenesKlebsiella pneumoniaePseudomonas aeruginosa, Providencia stuartii and Burkholderia pseudomallei. All of the screened bacteria, Bacillus subtilis indicated high level of biosurfactant production and was subsequently subjected to optimization for biosurfactant production. The emulsification index (E1%) due to change in temperature and pH on glucose/KN03 is 77.28, sucrose/KN03 is 59.80 and spent vegetable oil/KN03 is 57.16. The  mean value for hydrocarbon utilizing bacteria and total heterotrophic bacterial count were 1.5×105 cfu/g and 3.76×108 cfu/g for Opuama flow station, 5.8×104 cfu/g and 2.60×108 cfu/g for Ogini flow station, 2.80×105 cfu/g and 2.55×108 cfu/g for Oteghele river spill, 4.2×104 cfu/g and 3.04×108 cfu/g for Transforcados pipeline spill and 1.72×105 cfu/g and 2.75×108 cfu/g for Transfoecados right of way spill. Oteghele river spill had the highest concentration of crude oil utilization bacteria 2.80×105 cfu/g followed by Transforcados right of way spill 1.72×105 cfu/g while Opuama flow station had the highest concentration of heterotrophic bacteria 3.76×108 cfu/g. The performance of the pathogen for hemolytic reaction on blood agar, oil spreading on glass slide, blue plate agar reaction, emulsification index and lypolytic enzyme reaction indicated that they were significant at (p<0.05). There was significant difference in the physicochemical parameters at (p<0.05). The mean values of the pH range from 4.15d±0.1-5.75b±0.1, electrical conductivity 1179.61e±7.51- 2079.55b±1.45. Some of the heavy metals were higher in value when compared with the WHO standard. The structural metagenomics revealed eight top phyla; Proteobacteria, Actinobacteriota, Acidobacteriota, Bacteroidota, Planctomycetota, Firmicutes and Cloroflexi. The functional gene analysis revealed Carbohydrate metabolism, energy metaboilism, environmental information processing, degradation genes and various protein classes in the samples as contained in the KEGG and COG pipelines. Giving the findings of this study microorganisms found in petroleum hydrocarbon polluted soil were able to produce biosurfactants which helped in biodegradation.







TABLE OF CONTENTS

 

TITLE PAGE                                                                                                              i

DECLARATION                                                                                                        ii

CERTIFICATION                                                                                                      iii

DEDICATION                                                                                                            iv

ACKNOWLEDGEMENTS                                                                                        v

TABLE OF CONTENTS                                                                                           vi

LIST OF TABLES                                                                                                      xii

LIST OF FIGURES                                                                                                    xv

ABSTRACT                                                                                                               xix

                                                                                                                                               

CHAPTER 1: INTRODUCTION

1.1           Background of the Study                                                                                1

1.2           Justification                                                                                                    6

1.3           Aim and Objectives of the Study                                                                   6

1.4           Significance of the Study                                                                               7

CHAPTER 2: LITERATURE REVIEW

2.1        Exploration of Petroleum Hydrocarbon in Nigeria                                  8         

2.2        Origin of Petroleum Hydrocarbon                                                            8

2.3        Petroleum Hydrocarbon Formation in Various Depth Zones                   9         

2.4        Formation and Types of Kerogen                                                             10

2.5        Chemical Composition of Petroleum Hydrocarbon (crude oil)                  11

2.6         Crude Oil Classification                                                                          12       

2.7        Petroleum Biotechnology                                                                         13

2.8        Factors Affecting Hydrocarbon Degradation                                           13

2.9        Degradation Mechanism of Petroleum Hydrocarbon                               15

2.10         Biosurfactants Biotechnology                                                                 18

2.11        Biosurfactants Classification                                                                       19

2.12        Properties of Biosurfactant                                                                       27

2.13        Mechanisms of Interaction                                                                       27

2.14        Applications of Biosurfactants                                                                 30

2.14.1 Microbial Enhanced Oil Recovery                                                           30

2.14.2 Cleanup of Spilled Oil                                                                              30

2.14.3  Antimicrobial Activity                                                                             30

2.14.4  Medical and Therapeutic Applications                                                    30

2.14.5  Anti-adhesive Agents                                                                               31

2.14.6  Control of Disease and Plant Pathogen                                                    31

2.14.7  Applications in Food Processing                                                              31

2.15     Advantages of Biosurfactants                                                                   32

2.16     Disadvantages of Biosurfactants                                                              33

CHAPTER 3: MATERIALS AND METHODS

3.1       Study Site                                                                                                       35

3.2       Sample Collection                                                                                          35

3.2.1    Preparation of Soil Samples for Serial Dilution                                             38

3.3       Microbiological Analysis                                                                               38

3.3.1    Estimation of Hydrocarbon Utilizing Bacteria Count (HUB) of                 38

the Soil Samples A-E

 

3.3.2    Estimation of Total Heterotrophic Bacterial Count (THB) of                     39

the Soil Samples A-E

                                                                       

3.3.3    Characterization and Identification of Bacterial Isolates for                         39

 the Soil Samples A-E

                                                                       

3.4       Physicochemical Analysis                                                                              39

3.4.1    Determination of pH                                                                                       40

3.4.2    Determination of Conductivity and Redox Potential                                     40

3.4.3    Determination of Soil Total Nitrogen                                                            40

3.4.4    Determination of Total Phosphorus Content                                                  41

3.4.5    Determination of Percentage Total Organic Carbon                          41

3.4.6    Determination of Total Hydrocarbon Content                                               42

3.4.7    Determination of Total Petroleum Hydrocarbon                                           42

3.4.7.1 Preparation of Soil Sample Extracts                                                              43

3.4.8    Digestion of Soil Samples for Metal Analysis                                               43

3.4.9    Extraction of Cations in the Soil Samples                                                                                                      43

3.4.9.1 Determination of Exchangeable Cations                                                        44

3.4.10  Determination of Potassium and Sodium                                                                                                       44

3.4.11  Determination of Calcium and Magnesium                                                   44

3.4.12  Determination of Exchangeable Acidity                                                        45

3.4.13  Titration for Hydrogen ion (H+)                                                                     45

3.4.14  Determination of Effective Cation Exchange Capacity (ECEC)                         46

3.4.15  Determination of Soil Base Saturation                                                           46

3.4.16  Determination of Heavy Metals                                                                     46

3.5       Screening of Biosurfactant Producing Bacteria for the Soil Samples A- E  47       

3.5.1    Blood Agar Reaction (Haemolysis)                                                               47

3.5.2    Oil Spreading on Glass Plate                                                                          47

3.5.3    Blue Agar Plate Reaction                                                                               47

3.5.4    Measurement of Emulsification Index (E24)                                                  48

3.5.5    Lipolytic Enzyme Production                                                                         48

3.6       Optimization of Biosurfactant Producing Microorganisms Using                         48

Response Surface Methodology (RSM) for the Isolate

 

3.6.1    Inoculum Development of the Isolate Used for Optimization                        49

3.7       Metagenomic Analysis of the Soil Samples A-E                                           49       

3.7.1    Bacterial DNA Isolation from Samples                                                         50

3.7.2    Lysis of the Samples                                                                                       50

3.7.3    Binding to Column                                                                                         50

3.7.4    Column Wash                                                                                                 51

3.7.5    DNA Elution                                                                                                  51

3.7.6    DNA Amplification                                                                                        51

3.7.7    Metagenomic Sequencing of DNA                                                                 51

3.7.8    Functional Analysis of Sequence Reads                                                        52

3.8       Molecular Analysis                                                                                         52

3.8.1    Extraction of DNA                                                                                          53

3.8.2    PCR Reaction                                                                                                 54

3.9       Heat Map                                                                                                        54

3.10     Experimental Framework and Data Analysis                                                 55

CHAPTER 4: RESULTS AND DISCUSSION

4.1       Results                                                                                                            56

4.1.1    Microbiological Characteristics of the Soil Samples                                     56

4.1.2    Physicochemical Analysis of the Soil Samples (Sample A-E)                        60

4.1.3    Screening of Biosurfactant Producing Bacteria from the Soil Samples          64

4.1.4    Optimization Using Response Surface Methodology                                    66

4.1.5    Structural Metagenomics Analaysis of the Soil Samples                               79

4.1.6    Funtional Gene Analysis                                                                                123

4.1.7    PCR Reaction and Gel Electrophoresis                                                          123

4.2       Discussion of Findings                                                                                   162

4.2.1    Microbiological Analysis                                                                               162

4.2.2    Biosurfactant Producing Bacteria Analysis                                                    164

4.2.3    Optimization of Biosurfactant Producing Bacteria by (RSM)                        165

4.2.4    Physicochemical Analysis                                                                              166

4.2.5    Metals Analysis                                                                                              170

4.2.6    Structural Metagenomics Analysis                                                                 171

4.2.6    Functional Gene Analysis                                                                              181

CHAPTER 5: CONCLUSION AND RECOMMENDATIONS

5.1       Conclusion                                                                                                      184

5.2       Recommendation                                                                                           185

5.3       Contributions to Knowledge                                                                          186

REFERENCES

APPENDICES

 

 

 

 

 

 

 

LISTS OF TABLES

 

Table                                   Title                                                    page

2.1                   Classification of biosurfactant and important microorganisms          26

4.1                   Cell morphology and biochemical identification of isolates                        59

4.2                   Physicochemical properties of the different soil samples                        62

 (sample A-E)

 

4.3                   Metal properties of the different soil samples (sample A-E)                    63

4.4                   Performance of the bacterial isolate based on different screening         65

Methods

           

4.5                   Carbohydrate metabolism found in Opuama flow station sample 124

4.6                   Energy metabolism found in Opuama flow station sample                        125

4.7                   Environmental information processing found in Opuama flow     126

station

 

4.8                   Degradation genes found in Opuama flow station sample                        127

4.9                   Carbohydrate metabolism found in Ogini flow station sample 128

4.10                 Energy metabolism found in Ogini flow station sample                        129

4.11                 Environmental information processing found in Ogini flow                 130

station sample

 

4.12                 Degradation genes found in Ogini flow station sample                        131

4.13                 Carbohydrate metabolism found in Oteghele spill sample                        132

4.14                 Energy metabolism found in Oteghele spill sample                           133

4.15                 Environmental information processing found in Oteghele                         134

spill    

 

4.16                 Degradation genes found in Oteghele spill sample                            135

4.17                 Carbohydrate Metabolism found Transforcados pipeline                         136

spill sample

 

4.18                 Energy metabolism found in Transforcados pipeline spill sample 137

4.19                 Environmental information processing found in Transforcados 138

 pipeline spill sample

 

4.20                Degradation genes found in Transforcados pipeline spill sample 139

4.21                 Carbohydrate metabolism found in Transforcados right of                         140

way spill         

 

4.22                 Energy metabolism found in Transforcados right of way                         141

spill sample

 

4.23                 Environmental information processing found in Transforcados 142

                        right of way spill sample

 

4.24                Degradation genes found in Transforcados right of way spill sample143

4.25                 Cluster of orthology group (COG) class of Opuama flow                         144     

station sample

 

4.26                 Cluster of orthology group (COG) families of Opuama flow     145

station sample

 

4.27                 Phosphoribulokinase (PRK) of Opuama flow station sample 146

4.28                 Cluster of orthology group (COG) class of Ogini flow                         147

station sample

 

4.29                 Cluster of orthology group (COG) families of Ogini flow                         148

station sample

 

4.30                 Phosphoribulokinase (PRK) of Ogini flow station sample                        149

4.31                 Cluster of orthology group (COG) class of Oteghele                         150

spill sample    

 

4.32                 Cluster of orthology group (COG) family of Oteghele                         151

spill sample    

 

4.33                 Phosphoribulokinase (PRK) of Oteghele spill sample                        152

4.34                Cluster of orthology group (COG) class of Transforcados pipeline 153      spill sample

 

4.35                 Cluster of orthology group (COG) family of Transforcados             154

Pipieline spill sample

 

4.36                 Phosphoribulokinase (PRK) of Transforcados pipeline spill sample     155

4.37                 Cluster of orthology group (COG) class of Transforcados right of 156

 way spill sample

 

4.38                 Cluster of orthology group (COG) families of Transforcados right     157

of way spill sample

 

4.39                 Phosphoribulokinase (PRK) of Transforcados right of way                        158

                        spill sample    

 

 

 

 

 

LISTS OF FIGURES

 

Figure                             Title                                                    page

2.1                   Hydrocarbons degradation by microorganisms                                  17

2.2                   Examples of glycolipids and surfactin                                               22

2.3                   Reaction of surface tension and biosurfactant concentration 28

 

2.4                   Biosurfactants at water and air Interface                                            29

 

3.1                   Map of the study area                                                                         37

 

4.1                   Hydrocarbon utilizing bacterial count (HUB) of the                         57

 sampling sites (sample A-E)

 

4.2                   Total heterotrophic bacteria count (THB) of the sampling sites     58

(sample A-E)

 

4.3                   The distribution of Emulsification index (EI %) due to variation in      67

Temp and pH using glucose/KN03 as supplements

 

4.4                   The distribution of Emulsification index (EI %) due to variation          68

in Temp and pH using glucose/yeast extracts as supplements

 

4.5                   The distribution of Emulsification index (EI %) due to variation in      69

Temp and pH using glucose/soy bean source as supplements

 

4.6                   The distribution of Emulsification index (EI %) due to variation in      70

Temp and pH using glucose/locally prepared meat extract as

supplements

 

4.7                  The distribution of Emulsification index (EI %) due to variation in      71

Temp and pH using sucrose/KN03 as supplements

 

4.8                   The distribution of Emulsification index (EI %) due to variation in      72

Temp and pH using sucrose/yeast extract as supplements


4.9                   The distribution of Emulsification index (EI %) due to variation in      73

Temp and pH using sucrose/soy bean extract as supplements

 

4.10                 The distribution of Emulsification index (EI %) due to variation          74

in Temp and pH using sucrose/locally produced meat extract as supplements

 

4.11                 The distribution of Emulsification index (EI %) due to                         75

variation in Temp and pH using spent vegetable oil/KN03

as supplements

 

4.12                 The distribution of Emulsification index (EI %) due to variation          76

inTemp and pH using spent vegetable oil/yeast extract as

supplements

 

4.13                 The distribution of Emulsification index (EI %) due to variation          77

inTemp and pH using spent vegetable oil/soy beans source

as supplements

 

4.14                 The distribution of Emulsification index (EI %) due to variation          78

 inTemp and pH using spent vegetable oil/ locally prepared

meat extract as supplements

 

4.15                 Kingdom classification of Opuama flow station                                81

4.16                 Top phylum classification of Opuama flow station                           82

4.17                 Top class classification of Opuama flow station                                83

4.18                 Top order classification of Opuama flow station                               84

 

4.19                 Top family classification of Opuama flow station                             85

 

4.20                 Top genus classification of Opuama flow station                              86

 

4.21                 Top specie classification of Opuama flow station                             87

 

4.22                 Top kingdom classification of Ogini flow station                              90

4.23                 Top phylum classification of Ogini flow station                                91

4.24                 Top class classification of Ogini flow station                                    92

4.25                 Top order classification of Ogini flow station                                   93

4.26                 Top family classification of Ogini flow station                                 94

4.27                 Top genus classification of Ogini flow station                                   95

4.28                 Top species classification of Ogini flow station                                96

4.29                 Top kingdom classification of Oteghele spill                                    99

4.30                 Top phylum classification of Oteghele spill                                      100

4.31                 Top class classification of Oteghele spill                                           101

4.32                Top order classification of Oteghele spill                                          102

4.33                 Top family classification of Oteghele spill                                        103

4.34                 Top genus classification of Oteghele spill                                         104

4.35                 Top specie classification of Oteghele spill                                                     105

4.36                 Kingdom classification of Transforcados pipeline spill                        107

4.37                 Phylum classification of Transforcados pipeline spill                        108

4.38                 Class classification of Transforcados pipeline spill                           109

4.39                 Order classification of Transforcados pipeline spill                          110

4.40                 Family classification of Transforcados pipeline spill                         111

4.41                 Genus classification of Transforcados pipeline spill                          112

4.42                Specie classification of Transforcados pipeline spill                         113

4.43                  kingdom classification of transforcados right of way spill                        116

4.44                 Top phylum classification of transforcados right of way spill     117

4.45                 Top class classification of transforcados right of way spill                        118

4.46                 Top order classification of transforcados right of way spill                        119

4.47                 Top family classification of transforcados right of way spill                 120

4.48                 Top genus classification of Transforcados right of way spill                 121 4.49                      Top specie classification of Transforcados right of way spill         122

4.50                 Gel electrophoresis showing amplification bands of isolates                        159

4.51                 Heatmap of the top ten species from each sample (A to E)                        160

4.52                 Heatmap of the top ten genus from each sample (A to E)                        161

 

 

 

 


 

 

CHAPTER 1

INTRODUCTION


1.1           BACKGROUND OF THE STUDY

            World over, Overcoming the negative impacts on soil, air and water contamination is a problem for scientists and environmentalists (Imeh and Sunday, 2012).  According to Mehdi (2014) and Patowary et al. (2017), hydrocarbons are one of the environmental contaminants and the important source of energy in industry and day to day living. Their release in the environment, whether unintentionally or as a result of human activities has greatly destroyed the flora and fauna, polluted the water supply and destroyed human lives and properties. The discovery, extraction, refinement, transportation, and storage of petroleum and its byproducts also contribute to a serious environmental problem (Eze, 2010).  According to Das and Chandran (2011), the major causes of oil spills in Nigeria are corrosion of oil pipelines and storage tanks, pipeline sabotage and carelessness during oil production activities.

Also about 40,000 barrels of oil from Mobil platform in Akwa Ibom State in 1998 were spilled into the environment causing serious harm to the coastal environment (Eze, 2010). Hence, the oil-rich Niger Delta region of Nigeria is currently dealing with a significant ecological issue brought on by widespread crude oil contamination (Chikere et al., 2011).

All petroleum hydrocarbons originate from crude oil, which is made up of the fossilized remains of zooplankton and algae from ancient times that underwent catagenesis to form hydrocarbons. As the name implies, it is a heterogeneous and complex mixture of hydrocarbons made primarily of hydrocarbons like asphaltenes, resins, mono and polyaromatics, cycloalkanes, and aliphatic compounds (linear, branched, saturated, and unsaturated compounds). According to Joanna and Pawet (2018) and Arjoon and Speight (2020), crude oil is typically made up of 80% aromatic and saturated hydrocarbons. Petroleum hydrocarbon is primarily made up substituted hydrocarbons, with carbon making up 85%-90% and hydrogen accounting for 10%–14% of the mixture. The remaining components are non-hydrocarbon elements such as sulfur, nitrogen, vanadium, nickel, arsenic, lead and other metals in small quantities. Also Sodium chlorides, magnesium chloride and other metallic compounds like vanadium, phosphorus, lead, and nickel are part of it (Chaudhuri, 2011; Abdulatif, 2015).

Despite the economic advantages of the crude oil business, oil spillage affects and changes the composition of the soil's microbial community and biogeochemical cycles and has a significant detrimental impact on environmental quality and sustainable soil fertility (Milena et al., 2019). Cleanup methods are required in contaminated areas due to the harmful impacts of petroleum hydrocarbons on numerous ecosystem components. Burning, sinking, mechanical removal and the application of detergents are examples of physical and chemical cleanup techniques and these techniques do however, have drawbacks. The majority of them are pricey, while some merely move the oil to another site or possibly worsen environmental pollution (Eze, 2010).

Hydrocarbonoclastic bacteria are found in various habitats, including soils and water sediments and can degrade or alter petroleum hydrocarbons without causing any negative impacts. The bulk of natural hydrocarbon compounds can be broken down by microorganisms. Resins, asphaltenes, and polycyclic hydrocarbons with high molecular weights are less biodegradable. The nature of the majority of insoluble petroleum hydrocarbons inhibits this interaction, which is required for hydrocarbon uptake to occur by hydrocarbon degrading microorganisms using their substrate (Sampson, 2016).

Globally bioremediation is the use of the metabolic capacity of biological systems i.e. plants and microbes, to breakdown hazardous compounds into non harmful or harmless ones in the environment and so far have received much attention. This is accepted by the public for the cleanup of contaminated environment due to the fact that it is a natural method using the natures recycling and self-decontamination capabilities (Chikere et al., 2011). It is a favored treatment method for cleaning up hydrocarbon-contaminated soils and several studies have confirmed its efficacy and environmental friendliness in various geographical and ecological settings. It is also widely known that bacteria that use hydrocarbons are common in both polluted and unpolluted soil and that the availability of microorganisms with the required catabolic reaction is crucial for effective bioremediation. The three primary natural processes that remove hydrocarbons from the environment involve evaporation, photo-oxidation and microbial degradation. The reaction might take some time to stabilize contaminated areas. However, the development of low-cost, high-efficiency remediation techniques is therefore essential (Eze, 2010).

Chemically made surfactants are made to increase contaminant solubility; often they are toxic causing additional contamination to the environment. Similar qualities are shared by surface-active chemicals produced by microbes, although they are non-hazardous, biodegradable and produced at the polluted site. Surfactants and emulsifiers are released by bacteria that break down hydrocarbons to aid in the assimilation of these insoluble substrates. In contaminated areas, microorganisms that can emulsify and solubilize hydrophobic contaminants at site may have a distinct competitive advantage over rivals. As a result, it is often beneficial to isolate from such areas and the sites are usually abundant with the desired microorganisms with the required traits for both on site and off site bioremediation methods (Nwaguma et al., 2016). There are two primary categories of substances made by microorganisms: (1) biosurfactants that reduce surface tension at the air-water interface (2) bioemulsifiers, which lower interfacial tension between immiscible liquids or at the solid-liquid interface. Although biosurfactants typically have emulsifying abilities while bioemulsifiers do not always lower surface tension. According to Batista et al. (2006), biosurfactant is applied to improve oil recovery from wells, lessen viscosity of heavy oil, clean oil storage tanks, increase flow through pipelines, and stabilize fuel water-oil emulsions.

There is a high need for surfactants and was anticipated to have a global market between 30 to 64 billion US dollars in 2016 and 39 to 86 billion US dollars in 2021. The market for biosurfactants was 344068.40 tons in 2013 and is expected at yearly growth rate of 3–4% from 2014 to 2020, reaching 461991.67 tons. Revenue from biosurfactant market exceeded $1–8 billion in 2016 and is anticipated to increase to $2–6 billion by 2023, with the rhamnolipid market likely to grow by over 8% (Singh et al., 2018).

Surfactants contain amphiphilic molecules having polar and nonpolar moieties in one single molecule. They have a tendency to disperse liquids, lower surface tensions and cause solubility of non-polar compounds in polar solvents (Fenibo et al., 2019). Using biosurfactant producing microorganisms is a good strategy that is employed to accelerate the degradation of sites polluted with hydrocarbon.  Varieties of microorganisms produce biosurfactants with many chemical compositions, including glycolipids, fatty acids, lipopeptides and lipoproteins, phospholipids and neutral lipids. Some microbes produce biosurfactants into the growth medium during the hydrocarbon breakdown process, changing the cell surface's hydrophobicity in the process (Thavasi et al., 2011; Patowary et al., 2017; Al-Tamimi et al., 2019).

They are heterogeneous and produced by microorganisms. It is amphiphilic in nature and made up of a hydrophilic moiety and hydrophobic part causing their aggregation at surface between fluids with different polarities like water and hydrocarbons. The hydrophilic part contains monosaccharides or polysaccharides and proteins. The hydrophobic part comprises saturated, unsaturated, hydroxylated fatty acids and alcohols. It is made up two primary categories: biosurfactants and synthetic surfactants. Biosurfactants are formed by biological processes, as opposed to chemical reactions, which produced industrially (Nwaguma et al., 2016; Beulah et al., 2018). With their distinct characteristics like low toxicity, high biodegradability, good biocompatibility with eukaryotic organisms, effectiveness at a wider range of temperatures, pH values, and salinities, low irritancy, ability to be produced from renewable and inexpensive substrates and production  in a friendly conditions like low temperatures, biosurfactants have recently attracted much more interest than their chemical counterparts (Odalys et al., 2017).

            Biosurfactants producing microorganisms are widespread in the environment and can be found in both soil and water. Additionally, they can survive in a varying temperatures, pH and salinities and can be found in harsh situations (such as oil reserves). However, the best habitat for extensive biosurfactant production remains microbial communities that degrade hydrocarbons. Pseudomonas, Bacillus, Sphingomonas, Klebsiella, Actinobacteria, Halomonas, Alcanivorax and Acinetobacter are the key genera that typically dominate populations of hydrocarbon-degrading bacteria (Zhang et al., 2012; Nwaguma et al., 2016; Xu et al., 2018).

 

1.2       JUSTIFICATION

One of the challenges in the pollution of the environment is the release of petroleum hydrocarbons and their byproducts. Both industrialized and developing nations are focusing their attention on the cleanup of hydrocarbon pollution (Yanan et al., 2019). Petroleum compounds take much time to decompose because of their ability to bind to soil constituents. Since hydrocarbon is mostly a mixture of carbon and hydrogen, their spillage on soil brings about an imbalance in the carbon-nitrogen composition at the spill site. This results in a nitrogen shortage in polluted soil and inhibits bacterial growth and the uptake of carbon sources (Olajire and Essien, 2014). Through the use of various microorganisms that may use hydrocarbons as food, bioremediation has the potential to degrade, modify, remove, immobilize or detoxify harmful compounds existing in the earth's biospheres (Xu et al., 2018).

Total degradation, mineralization, sequestration of toxic contaminants and microbial activity result in the cleaning of the environment (Seema and Ajinath, 2018). Traditional physical and/or chemical treatments use a lot of energy, cost a lot of money, and leave behind residues that are harmful to the biota. According to Vijavakumar and Saravanan (2015), the properties of microbial surfactants include surface activity, tolerance to pH, temperature, and ionic strength, biodegradability, low toxicity, emulsifying and demulsifying ability, and antimicrobial activity.


1.3       AIM AND OBJECTIVES

This research is aimed at evaluating the physicochemical parameters, biosurfactant production and metagenomic analysis of hydrocarbon polluted soil in parts of Delta State Nigeria.

 

 

1.4       SPECIFIC OBJECTIVES

These include to:

1.     Estimate heterotrophic bacteria and hydrocarbon utilizing bacteria

2.     Screen and characterize bio-surfactant producing bacteria from hydrocarbon contaminated soil

3.     Optimize bio-surfactants production from the isolated bacterial species

4.     Determine the physicochemical characteristics of the various soil samples

5.     Determine the total petroleum hydrocarbon and heavy metals of the soil samples

6.     Apply metagenomic tools to examine the various microbial communities in the soil samples

7.     Determine the functional gene analysis of the microbial communities, including the reaction of the microorganisms in degradation of petroleum hydrocarbon

 

1.5       SIGNIFICANCE OF THE STUDY

            The Significance of the study was to isolate microorganisms capable of degrading hydrocarbons contaminating the environment. These organisms were observed to produce biosurfactant enhancing the degradation of petroleum htdrocarbons in the studied sites.

 

 

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